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h he simple procedure used here to find a correlation for G ~ / R T would no doubt be improved by a regression / procedure that determines the values of Azl and AI2 that minimize the sumof squares of theresiduals S ( G ~R T )

Figure 129 shows plots of In yi based on experimental measurements for six binary systems at 32315 K (50 C), illustrating the variety of behavior that is observed Note in every case that as xi + 1, In yi -+ 0 with zero slope Usually (but not always) the infinite-dilution activity coefficient is an extreme value Comparison of these graphs with those of Fig 114 indicates that the In yi generally have the same sign as G E That is, positive G Eimplies activity coefficients greater than unity and negative G E implies activity coefficients less than unity, at least over most of the composition range

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Our modern theory of the atom describes it as an electrically neutral sphere with a tiny nucleus at the center, which holds the positively charged protons and the neutral neutrons The negatively charged electrons move around the nucleus in complex paths, all of which comprise the electron cloud Table 51 summarizes the properties of the three fundamental subatomic particles: Table 51 The Three Fundamental Subatomic Particles

s ~A Barker,Austral J Chem, vol 6, pp 207-210, 1953

LOMBARDI RULE #2

Figure 129 Logarithms of the activity coefficients at 32315 K (50 C) for six binary liquid systems: (a) chloroform(l)ln-heptane(2); (b) acetone(l)/methanol(2); ( c ) acetone(l)lchloroform(2); ( d ) ethanol(1)ln-heptane(2); (e) ethanol(l)/chloroform(2); ( f ) ethanol(l)/water(2)

In general G E /RT is a function of T, P, and composition, but for liquids at low to moderate pressures it is a very weak function of P Therefore the pressure dependence of activity coefficients is usually neglected Thus, for data at constant T :

Demand autonomy What do you absolutely have to control, to make your job possible If you can t get that degree of autonomy, you can t succeed

1+ 0 1

,XN)

(const T )

The Margules equation, Eq (129), is an example of this functionality A number of other equations are in common use for correlation of activity coefficients For binary systems (species 1 and 2) the function most often represented by an equation is

I ve included many of my father s thoughts on this subject because it seems clear to me that by striking the right deal up front, he gave himself enormous latitude to make changes on the scale, and of the scope, that he was contemplating This was truly a case in which a business turnaround was needed (It s hard to get much lower than 1 10 1!) The Packers executive committee had consciously gone out and hired what would today be called a turnaround artist Lombardi had demanded, and the board had agreed to cede, sufficient authority to make things happen Of course, these are the specifics of a particular situation I think the generalizations behind the specifics, however, are still meaningful: Develop a clear sense of the right opportunity Understand your bargaining position Bargain for autonomy, especially if you re planning big changes Give yourself enough elbowroom to survive the inevitable missteps of the initial phase of your new situation I should also point out that my father was not demanding unchecked, unlimited authority for himself That would have been unrealistic Despite his carefully engineered autonomy, he still lived within two hierarchies: the Packer organization and the NFL Although he sometimes had disagreements with representatives of both of these organizations, he usually followed the rules and conducted himself as a subordinate when such conduct was appropriate

(const T ) Since x2 = 1 - X I , mole fraction X I serves as the single independent variable An equivalent power series with certain advantages is known as the RedlicWKister e ~ p a n s i o n : ~

1007 1009 5486 10 4

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